Cryogenic Buffer-gas Cooled Beams

Schematic of the inside of the CBGB cell, with the buffer gas flowing in from the left, the laser ablation (forming the clusters) at the bottom, and the cell exit and probe QCL laser on the right. 

A Cryogenic Buffer-Gas Beam (CBGB) consists of a cold, inert gas (such as neon or helium) flowing in a specific direction (often through a CBGB cell), with some species of interest entrained in the flowing gas. Many species of interest (such as reactive molecules, clusters, etc.) do not remain gaseous at the temperatures desirable for further scientific study (~4 – 30 K). However, if these species are entrained in a flowing, inert gas that can be held at these temperatures, the species of interest can be cooled to these low temperatures and still remain in the gas phase for further study. In our lab, we are working on producing carbon clusters and metal oxide clusters, produced via laser ablation of a solid target and then cooled to ~25 K in a neon buffer gas beam. These types of clusters have relevance to many different fields of research, including astronomical and interstellar physics and chemistry, combustion chemistry and soot formation, and catalysis, just to name a few.