TY - JOUR AU - Daniil Lukin AU - Alexander White AU - Rahul Trivedi AU - Melissa Guidry AU - Naoya Morioka AU - Charles Babin AU - Öney Soykal AU - Jawad Ul-Hassan AU - Nguyen Son AU - Takeshi Ohshima AU - Praful Vasireddy AU - Mamdouh Nasr AU - Shuo Sun AU - Jean-Philippe MacLean AU - Constantin Dory AU - Emilio Nanni AU - Jörg Wrachtrup AU - Florian Kaiser AU - Jelena Vučković AB - The ability to shape photon emission facilitates strong photon-mediated interactions between disparate physical systems, thereby enabling applications in quantum information processing, simulation and communication. Spectral control in solid state platforms such as color centers, rare earth ions, and quantum dots is particularly attractive for realizing such applications on-chip. Here we propose the use of frequency-modulated optical transitions for spectral engineering of single photon emission. Using a scattering-matrix formalism, we find that a two-level system, when modulated faster than its optical lifetime, can be treated as a single-photon source with a widely reconfigurable photon spectrum that is amenable to standard numerical optimization techniques. To enable the experimental demonstration of this spectral control scheme, we investigate the Stark tuning properties of the silicon vacancy in silicon carbide, a color center with promise for optical quantum information processing technologies. We find that the silicon vacancy possesses excellent spectral stability and tuning characteristics, allowing us to probe its fast modulation regime, observe the theoretically-predicted two-photon correlations, and demonstrate spectral engineering. Our results suggest that frequency modulation is a powerful technique for the generation of new light states with unprecedented control over the spectral and temporal properties of single photons. BT - npj Quantum Information DO - 10.1038/s41534-020-00310-0 IS - 1 N2 - The ability to shape photon emission facilitates strong photon-mediated interactions between disparate physical systems, thereby enabling applications in quantum information processing, simulation and communication. Spectral control in solid state platforms such as color centers, rare earth ions, and quantum dots is particularly attractive for realizing such applications on-chip. Here we propose the use of frequency-modulated optical transitions for spectral engineering of single photon emission. Using a scattering-matrix formalism, we find that a two-level system, when modulated faster than its optical lifetime, can be treated as a single-photon source with a widely reconfigurable photon spectrum that is amenable to standard numerical optimization techniques. To enable the experimental demonstration of this spectral control scheme, we investigate the Stark tuning properties of the silicon vacancy in silicon carbide, a color center with promise for optical quantum information processing technologies. We find that the silicon vacancy possesses excellent spectral stability and tuning characteristics, allowing us to probe its fast modulation regime, observe the theoretically-predicted two-photon correlations, and demonstrate spectral engineering. Our results suggest that frequency modulation is a powerful technique for the generation of new light states with unprecedented control over the spectral and temporal properties of single photons. PB - Springer Science and Business Media LLC PY - 2020 EP - 80 T2 - npj Quantum Information TI - Spectrally reconfigurable quantum emitters enabled by optimized fast modulation VL - 6 SN - 2056-6387 ER -